My favorite is Gankutsuou the Count of Monte Cristo http://www.anime-planet.com/anime/gankutsuou-the-c... Everything about this anime is perfect. It has a lot of suspense and mystery, interesting characters, great music and best of all a beautiful unique art style that is very enthralling to the viewers.
Update:@Lorna I really like Kaiji too I'm actually watching it right now.
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Kaiji by far. It was just so fun and suspenseful to watch, and I was always excited to see how Kaiji would get himself out of each situation he was in. I also love the fkmt art style, it's ugly at first, but it starts to get cute as it grows on you.
Monster. Not only is my favorite seinen anime, but it's my favorite anime in general.
Yep, Gankutsuou was pretty great. There are so many great seinen anime I've enjoyed that I don't even know what I'd pick as my #2. Even narrowing them down to a top 10 list would be pretty tough.
Bokurano. It's perfection when it comes to psychological aspects. These kid are only eleven-ish and they know their going to die, because if the fight they die but if they don't they die anyway along with the rest of the world. It's also made worse when you find out that every time they win a battle they are wiping out a whole universes existence and they have to choose whether it's really right to keep going.
Btooom! and Cannan.